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- W2063706701 abstract "In the course of an attempt to investigate experimentally the hypothesis that acetylene is the last stable precursor to carbon in rich premixed hydrocarbon flames, the isotopic composition of the carbon (or soot) formed in closed bomb explosion flames of propane-2-13C has been studied. The results show definitely that carbon does not arise preferentially from a two-carbon piece of the fuel molecule; that is, if acetylene polymerization-decomposition is the actual mechanism of carbon formation, then the acetylene does not contain a carbon pair of the propane and must arise by a process more complicated than simple degradation of the fuel. Isotopic analyses of gaseous products show that methane and carbon monoxide come equally from all three carbon atoms of the propane, and that the acetylene remaining does in fact contain a nearly random isotope distribution, such as would result from its synthesis in the flame from single-carbon radicals. The composition of other products is given. As a test of whether carbon monoxide participates in carbon formation in hydrocarbon flames, possibly by reaction with existing nuclei, 13CO was burnt in an ordinary propane flame. Neither the carbon collected nor the gaseous products, except carbon dioxide, contained 13C in significant excess over the natural abundance." @default.
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- W2063706701 date "1957-12-01" @default.
- W2063706701 modified "2023-09-23" @default.
- W2063706701 title "An isotopic tracer study of carbon formation in hydrocarbon flames" @default.
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- W2063706701 doi "https://doi.org/10.1016/0010-2180(57)90004-4" @default.
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