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- W2063762457 abstract "Abstract Dissociative multiple photoionization of the bromine, the iodine monobromide, and the iodine molecules in the Br(3d,3p,3s) and I(4d,4p,4s,3d,3p) inner-shell regions has been studied by using time-of-flight (TOF) mass spectrometry coupled to synchrotron radiation in the ranges of 90∼978 eV for Br 2 , 60∼133 eV for IBr, and 86∼998 eV for I 2 . Total photoion and photoion–photoion coincidence (PIPICO) yields have been recorded as functions of the photon energy. Here, giant shape resonances have been observed beyond the thresholds of the inner-shells owing to the Br(3d 10 )→Br(3d 9 ϵ f), I(4d 10 )→I(4d 9 ϵ f), and I(3d 10 )→I(3d 9 ϵ f) transitions. The dissociation processes of the multiply charged parent ions have also been evaluated from variations of photoelectron–photoion coincidence (PEPICO) and PIPICO spectra with the photon energy. From each Br(3p 3/2 ) (189.9 eV) and I(4p 3/2 ) threshold (129.9 eV), quintuple ionization of the molecules begins to play important roles in the photoionization, subsequently yielding ion pairs of X 3+ –X 2+ (X=Br, I). From the I(3d 5/2 ) threshold (627.3 eV), loss of six electrons from iodine molecule additionally begins to play a minor role in the multiple photoionization, giving rise to the formation of ion pairs of either I 3+ –I 3+ or I 4+ –I 2+ . A direct comparison of the strengths and the ranges of the I(4d) and Br(3d) giant resonances was successfully made from dissociative photoionization of IBr. Over the entire energy range examined, 60 E" @default.
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- W2063762457 date "2002-12-01" @default.
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- W2063762457 title "Dissociative multiple photoionization of Br2, IBr, and I2 in the VUV and X-ray regions: a comparative study of the inner-shell processes involving Br(3d,3p,3s) and I(4d,4p,4s,3d,3p)" @default.
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- W2063762457 doi "https://doi.org/10.1016/s0368-2048(02)00162-7" @default.
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