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• W2063973792 abstract "The effects of non-equilibrium charge screening in mixtures of oppositely charged interacting molecules on surfaces are analyzed in a closed system. The dynamics of charge screening and the strong deviation from the standard Debye-Hückel theory are demonstrated via a new formalism based on computing radial distribution functions suited for analyzing both short-range and long-range spacial ordering effects. At long distances the inhomogeneous molecular distribution is limited by diffusion, whereas at short distances (of the order of several coordination spheres) by a balance of short-range (Lennard-Jones) and long-range (Coulomb) interactions. The non-equilibrium charge screening effects in transient pattern formation are further quantified. It is demonstrated that the use of screened potentials, in the spirit of the Debye-Hückel theory, leads to qualitatively incorrect results." @default.
• W2063973792 created "2016-06-24" @default.
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• W2063973792 date "2011-07-20" @default.
• W2063973792 modified "2023-10-16" @default.
• W2063973792 title "The non-equilibrium charge screening effects in diffusion-driven systems with pattern formation" @default.
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• W2063973792 doi "https://doi.org/10.1063/1.3613622" @default.
• W2063973792 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21787018" @default.
• W2063973792 hasPublicationYear "2011" @default.
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