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• W2063980596 abstract "A theory of coherent excitation of a localized state on an adatom by two-photon photoemission spectroscopy (TR-2PPE) is presented within a microscopic model and the time-dependent formalism. Coherent oscillation and incoherent population decay of the excitation are obtained, and are shown to attain well-defined lifetime constants only in the long-delay limit. In addition, we have found a competing excitation channel via electron transfer. The theory is applied to Cs/Cu (111), which reproduces a few qualitative features observed in recent experiments. The effect of atomic motion on the 2PPE spectra, which manifests dominantly as a redshift in the spectrum, has been analysed." @default.
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• W2063980596 date "2002-07-30" @default.
• W2063980596 modified "2023-09-24" @default.
• W2063980596 title "Coherence and Decoherence of a Localized Excitation on a Surface Adatom" @default.
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• W2063980596 doi "https://doi.org/10.1088/0256-307x/19/8/350" @default.
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