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- W2063996884 abstract "Mesoporous silicates (MCM-41 and Al-containing MCM-41) were applied to catalyst supports for liquid-phase benzene oxidation paying attention to their remarkable features, such as large surface area, ordered mesopores and high thermal stability. The MCM-41-supported Cu catalysts were prepared by the method of impregnation (Cu/MCM-41) and ion-exchange treatment (Cu–Na·MCM-41, Cu–H·MCM-41). The liquid-phase oxygenation of benzene to phenol over the MCM-41-supported Cu catalysts was studied using molecular oxygen as an oxidant and ascorbic acid as a reducing reagent for the Cu species. The MCM-41-supported Cu catalysts, particularly the Cu ion-exchanged H·MCM-41 (Cu–H·MCM-41), were more active than the corresponding Cu catalysts supported on SiO2, TiO2, MgO, NaZSM-5, NaY, or KL zeolites. The accumulation of hydrogen peroxide (H2O2) was confirmed during the liquid-phase oxidation of benzene catalyzed by the Cu-supported MCM-41." @default.
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- W2063996884 date "1998-10-01" @default.
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- W2063996884 title "Formation of Cu-supported mesoporous silicates and aluminosilicates and liquid-phase oxidation of benzene catalyzed by the Cu-mesoporous silicates and aluminosilicates" @default.
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- W2063996884 doi "https://doi.org/10.1016/s1381-1169(97)00298-7" @default.
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