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• W2064031912 abstract "ESR study on monodispersed palladium nanoparticles with the mean diameters of 25 Å corresponding to the “magic atom number” of 561 atoms (five-shell nanoparticle) and smaller than 25 Å (22 and 23 Å) was carried out to investigate their electronic structures. Two broad absorption peaks corresponding to ΔS = 1 and 2 and a sharp one with ΔS = 1 were observed in the ESR spectra of palladium nanoparticles. The broad and strongest spectrum with ΔS = 1 may arise from the spin on the large orbital moment state of the nanoparticles. The relatively strong second harmonic spectrum with ΔS = 2 is characteristic of the nanoparticles, and its low-field shift compared with bulk palladium implies the existence of the effective field from the orbital moment of the electron. On the other hand, the sharp ESR signal with ΔS = 1 may be derived from the nanoparticles that have the electronic structure with one s-state electron outside the closed electron shell core with the “magic atom number”." @default.
• W2064031912 created "2016-06-24" @default.
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• W2064031912 date "1997-07-01" @default.
• W2064031912 modified "2023-10-17" @default.
• W2064031912 title "ESR Study on Palladium Nanoparticles" @default.
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• W2064031912 doi "https://doi.org/10.1021/jp970599y" @default.
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