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• W2064354310 abstract "A series of four dichromophoric rigid macrocycles 6a−6d, two with diphenyloligothiophene chromophores, the other two with more electron-rich diphenyl-EDOT or diphenyl-bis-EDOT chromophores, have been synthesized. The absorption spectrum of the diphenyl-bis-EDOT based macrocycle 6d displayed the most pronounced vibronic resolution with a well-resolved 0−0 transition, indicating a fully planarized geometry of the diphenyl-bis-EDOT chromophores. The 1H NMR spectra of the macrocycles displayed weak to moderate chemical shifts of characteristic signals upon addition of π-conjugated oligonitro-9-fluorenone acceptors. X-ray single-crystal analysis showed that columnar π-stacked donor/acceptor complexes are formed with the stacks composed of alternating donor and acceptor molecules. The stoichiometry of the crystalline, dark-colored complexes was found to be 1:1 by elemental analysis and integration of the 1H NMR peaks. The complex formation is accompanied by remarkably large Stern−Volmer constants of fluorescence quenching." @default.
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• W2064354310 date "2006-12-01" @default.
• W2064354310 modified "2023-10-18" @default.
• W2064354310 title "Diphenyloligothiophene-Based Dichromophoric Macrocycles and Their Ability to Form Donor/Acceptor Complexes" @default.
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• W2064354310 doi "https://doi.org/10.1021/jp065443p" @default.
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