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• W2064366926 abstract "The appraisal of an association of the VLEED technique and the new models for oxygen chemisorption [Vacuum, J. Phys. Chem. Solids, in press] motivated and enabled us to seek physical insight into the dynamics of the O-Cu(001) surface reaction. It is shown that the discrete stages revealed by exposure-resolved VLEED can be quantified and interpreted by the process dominated by three bonding parameters: First, one Goldschmidt-contraction ionic bond forms between the O adsorbate and a Cu atom on the surface accompanying the vacating of the missing row. Second, another contracting ionic bond follows between the O and a Cu in the substrate; as a result, the oxygen buckles into the bulk. Then, the ionic bond angle increases leading to the relaxation, and finally, interaction develops between the non-bonding states of the oxygen and the lone-pair-induced metal dipoles." @default.
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• W2064366926 creator A5083679415 @default.
• W2064366926 date "1997-06-01" @default.
• W2064366926 modified "2023-10-18" @default.
• W2064366926 title "Exposure-resolved VLEED from the O-Cu(001): bonding dynamics" @default.
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• W2064366926 doi "https://doi.org/10.1016/s0042-207x(97)00007-9" @default.
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