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- W2064497306 abstract "A bstract : We compared time‐resolved Raman spectroscopic measurements of CH 4 ‐saturated aqueous solution with CH 4 hydrate crystal formed from the same solution. At 287.1 K and 6.6 MPa the C‐H stretching mode for CH 4 molecules in the solution (ν sol = 2911.7 cm −1 ) was intermediate between that in the large cage (ν L = 2905.1 cm −1 ) and that in the small cage (ν S = 2914.1 cm −1 ), thus indicating an intermediate molecular environment. Comparison of these results with previous work on the CO 2 ‐H 2 O system indicated that water molecules in the type‐I small‐cage‐like structure surrounded CH 4 molecules in the solution. Furthermore, the free energy barrier for CH 4 hydrate nucleation is likely to be formation of the large cage structure, which is probably larger than that for CO 2 hydrate formation." @default.
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- W2064497306 date "2000-01-01" @default.
- W2064497306 modified "2023-10-14" @default.
- W2064497306 title "In Situ Observations of Methane Hydrate Formation Mechanisms by Raman Spectroscopy" @default.
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- W2064497306 doi "https://doi.org/10.1111/j.1749-6632.2000.tb06814.x" @default.
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