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• W2064762114 abstract "The mononuclear Co(II) complex CoBr (dmph = 2,9-dimethyl-1,10-phenanthroline) was obtained and X-ray structurally characterized as a distorted tetrahedron environment that is responsible for the moderately strong positive anisotropy of high spin Co(II). In combination with variable-field magnetic susceptibility data at low temperature, high-field electron paramagnetic resonance (HF-EPR) spectroscopy reveals the presence of easy-plane anisotropy (D > 0) in complex CoBr. Slow magnetic relaxation effects were observed for CoBr in the presence of a dc magnetic field. At very low temperatures, ac magnetic susceptibility data show the magnetic relaxation time, τ, to be temperature-independent, while above 2.4 K thermally activated Arrhenius behavior is dominated with Ueff = 22.8(8) cm(-1) and τ0 = 3.7(5) × 10(-10) s. Upon dilution of the complex within a matrix of the isomorphous compound ZnBr, ac susceptibility data reveal the individual molecular nature of the slow magnetic relaxation and indicate that the quantum tunneling pathway observed at low temperatures is likely mediated by intermolecular dipolar interactions." @default.
• W2064762114 created "2016-06-24" @default.
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• W2064762114 date "2013-01-01" @default.
• W2064762114 modified "2023-10-18" @default.
• W2064762114 title "Field-induced slow relaxation of magnetization in a tetrahedral Co(ii) complex with easy plane anisotropy" @default.
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• W2064762114 doi "https://doi.org/10.1039/c3dt51801a" @default.
• W2064762114 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24002675" @default.
• W2064762114 hasPublicationYear "2013" @default.
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