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• W2064778872 abstract "We present a single-molecule study unraveling the effect of static disorder on the vibrational-assisted ultrafast exciton dynamics in multichromophoric systems. For every single complex, we probe the initial exciton relaxation process by an ultrafast pump-probe approach and the coupling to vibrational modes by emission spectra, while fluorescence lifetime analysis measures the amount of static disorder. Exploiting the wide range of disorder found from complex to complex, we demonstrate that static disorder accelerates the dephasing and energy relaxation rate of the exciton." @default.
• W2064778872 created "2016-06-24" @default.
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• W2064778872 date "2006-11-20" @default.
• W2064778872 modified "2023-10-18" @default.
• W2064778872 title "Effect of Disorder on Ultrafast Exciton Dynamics Probed by Single Molecule Spectroscopy" @default.
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• W2064778872 doi "https://doi.org/10.1103/physrevlett.97.216403" @default.
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