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- W2064904020 abstract "To resolve discrepancies between the existing low temperature ΔḠO2 data for solid solution mixed (U, Pu)-oxide nuclear fuel material, additional measurements have been performed on U0.75Pu0.25O2±x employing a combined thermogravimetric (TGA) and solid-electrolyte galvanic cell technique. These measurements, which were performed at temperatures between 800 and 1000°C, and for O : M ratios in the range 1.940 to 2.028, are reasonably self-consistent and show good agreement with the results of previous TGA measurements. However, they do not corroborate the earlier EMF cell measurements of Markin and McIver. Possible explanations for errors in these earlier EMF cell results are examined. The new results indicate that the ΔḠO2 of stoichiometric mixed oxide at typical outer surface fuel temperatures is close to −100 kcal/mol O2 (−419 kJ/mol O2). Attempts have been made to fit the new ΔḠO2 data to two equations derived from recent defect models, and it is shown that neither equation accurately represents the experimental po2 −x data over more than a short range of x." @default.
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- W2064904020 date "1979-06-01" @default.
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- W2064904020 title "The oxygen potential of near- and non-stoichiometric urania-25 mol% plutonia solid solutions: A comparison of thermogravimetric and galvanic cell measurements" @default.
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- W2064904020 doi "https://doi.org/10.1016/0022-3115(79)90040-0" @default.
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