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• W2065117329 abstract "Optical spectra and the magnetism between 4.2 and 300 K of the uranates(V) Li7UO6, Li3UO4, LiUO3, NaUO3, KUO3, the neptunates(VI) Ba3NpO6, Li4NpO5, Na2NpO4 and the plutanate(VII) Li5PuO6 are reported. The spectra were assigned to transitions between the ground state Γ7(a2) and the excited states Γ8(t2), Γ7′(t2), Γ8′(t1) and Γ6(t1) of the (Sf)1 configuration in a cubic or tetragonal symmetry. The magnetic susceptibility as a function of temperature was calculated, in conjunction with the spectra, on the basis of a ligand field of cubic or tetragonal symmetry. For Li7UO6, e.g., the physical data are well reproduced, assuming a slight tetragonal distortion, with the parameter values Δ = 4604, Θ = 7099, δ = 145, ξ = 1870 cm−, k = 1.0, k′ = 0.85 in combination with a correction term TIP* = 10 × 10−6 cgs mol−1 for the magnetic susceptibility. Similar results were obtained for the other uranates(V) as well as for Ba3NpO6. For Li4NpO5, the parameter values Δ = 9141, Θ = 3527, δ = 800, ξ = 1800 cm−1, k = 0.80, k = 1.0 were employed in conjunction with TIP* = 125 × 10−6 egs mol−1. An analogous approach was followed for Na2NpO4 and Li5PuO6. A magnetic transition to long-range order of the ferromagnetic type has been observed for LiUO3 at Tc = 16.9 K and for NaUO3 at Tc = 31.1 K. Anomalous magnetic behaviour at low temperature is also indicated for KUO3, Li4NpO5 and Na2NpO4." @default.
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• W2065117329 date "1980-11-01" @default.
• W2065117329 modified "2023-10-16" @default.
• W2065117329 title "Optical spectra and magnetism between 4.2 and 300 K for some alkali metal and alkaline earth metal uranates(V), neptunates(VI) and a plutonate(VII)" @default.
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• W2065117329 doi "https://doi.org/10.1016/0301-0104(80)87067-4" @default.
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