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- W2065298114 abstract "A microarray of electrochemiluminescent (ECL) nanosensors for remote detection is reported. Such nanosensor arrays were created on the distal face of coherent optical fibre bundles by adapting near-field optical probe and nanoelectrode methodologies. The fabrication process allows the production of high-density microarrays of nanosensors where each optical aperture is surrounded by a gold nanoring electrode. The initial architecture of the optical fibre bundle is retained and thus the microarray keeps its imaging properties. The electrochemical response of the array displays a steady-state current. This feature indicates that the nanoelectrodes forming the array can be considered as diffusively independent. In other words, each ring-shaped electrode of the array probes electrochemically a different micro-environment. We also show that this microdevice can be used as an ECL nanosensor microarray. Indeed, ECL light is initiated by the gold nanoring electrode in the presence of a co-reactant biospecies, NADH. A fraction of the isotropically electrochemically generated light is collected by the same aperture, transmitted by the corresponding fibre core and eventually imaged by a CCD camera. The gold coating therefore acts as an electrode material and also to confine the ECL light in each etched core. Such nanostructured microdevice integrates ECL-light generation, collection and imaging in a microarray format." @default.
- W2065298114 created "2016-06-24" @default.
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- W2065298114 date "2006-04-13" @default.
- W2065298114 modified "2023-10-13" @default.
- W2065298114 title "Development of an ordered microarray of electrochemiluminescent nanosensors" @default.
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- W2065298114 doi "https://doi.org/10.1088/0957-0233/17/5/s45" @default.
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