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- W2065394940 abstract "An approximate rate equation for a dense-gas chemical reaction of the type A + B ⇌ C + D is derived from first; principles starting from a hamiltonian formulated in terms of the field operators of the species. The rate equation considers the reactive binary collisions together with the spatial correlations between the molecules of the reactive pair the correlations being produced by the collisions of the surrounding molecules with the molecules of this pair. Simplifying the reaction mechanism the rate constants are written as a product of the dilute-gas rate constants times the pair distribution function which accounts for the spatial correlation." @default.
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- W2065394940 date "1980-12-01" @default.
- W2065394940 modified "2023-09-26" @default.
- W2065394940 title "On the influence of spatial correlations on the rate of chemical reactions in dense gases. I. Quantum statistical theory" @default.
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- W2065394940 doi "https://doi.org/10.1016/0301-0104(80)85131-7" @default.
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