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• W2065441630 abstract "Carbon monoxide (CO) is a major component in typical feed gases for solid oxide fuel cells (SOFC). This paper presents a combined modeling and experimental analysis of electrochemical CO oxidation on Ni/YSZ patterned model anodes. A computational model representing the coupled behavior of heterogeneous chemistry and electrochemistry in terms of elementary reactions is developed, which allows for a quantitative description of electrochemical impedance spectra and current–voltage behavior. Excellent agreement between model and experiment was achieved for the complete experimental data set, which covers a wide range of CO/CO2/N2 gas compositions (4.0 × 102 Pa ≤ pCO ≤ 5.1 × 104 Pa and 9.5 × 102 Pa ≤ pCO2 ≤ 9.2 × 104 Pa) and operating temperatures (973 K ≤ T ≤ 1073 K). In the framework of the presented model a direct mechanistic interpretation of the experimentally observed electrochemical characteristics is obtained." @default.
• W2065441630 created "2016-06-24" @default.
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• W2065441630 date "2012-01-01" @default.
• W2065441630 modified "2023-09-27" @default.
• W2065441630 title "Elementary kinetic modeling and experimental validation of electrochemical CO oxidation on Ni/YSZ pattern anodes" @default.
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• W2065441630 doi "https://doi.org/10.1016/j.electacta.2011.11.020" @default.
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