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- W2065458043 abstract "The rotational correlation times of C2D2 and CO2 in liquid n-heptane were determined by infrared spectroscopy as a function of temperature. On the basis of the present and other preceding data we propose an interpretation of the rotational motion of small molecules in inert solvents. In this free-volume model the probe molecule is able to rotate freely during a time interval x and is in hydrodynamic interaction with the solvent during the rest (1 − x). The correlation time of the angular momentum τJ is, under these conditions, simply given by a linear relation τJ = x(τJ)coll + (1 − x)(τJ)hydro. This model fits very well the experimental data with a value of x consistent with its physical definition." @default.
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- W2065458043 date "1985-12-01" @default.
- W2065458043 modified "2023-09-27" @default.
- W2065458043 title "Rotation of small molecules in liquids. A free-volume model combining collective and collisional effects" @default.
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- W2065458043 doi "https://doi.org/10.1016/0301-0104(85)85011-4" @default.
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