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- W2065542858 abstract "Cobalt(0) nanoparticles supported on graphene have been synthesized via a one-step in situ procedure, using the mixture of ammonia borane (AB) and sodium borohydride (NaBH4) as the reducing agents under ambient temperature. Compared with NaBH4, the as-prepared Co/graphene NPs which reduced by the mixture of NaBH4/AB exhibit superior catalytic activity towards the hydrolytic dehydrogenation of AB. A kinetic study shows that the catalytic hydrolysis of AB is first order with respect to the concentration of the as as-synthesized NPs. The turnover frequency (TOF) is 13.8 mol H2 min−1 (mol Co)−1, which is higher than most of the non-noble metal catalysts, and even noble-metal based NPs. The activation energy has been measured to be 32.75 kJ mol−1, which is lower than many reported values for the catalytic hydrolytic dehydrogenation of ammonia borane." @default.
- W2065542858 created "2016-06-24" @default.
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- W2065542858 date "2014-01-01" @default.
- W2065542858 modified "2023-10-10" @default.
- W2065542858 title "Graphene supported cobalt(0) nanoparticles for hydrolysis of ammonia borane" @default.
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- W2065542858 doi "https://doi.org/10.1016/j.matlet.2013.10.039" @default.
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