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• W2065575498 abstract "Boron is carbon’s neighbour in the periodic table and has similar valence orbitals. However, boron cannot form graphene-like structures with a honeycomb hexagonal framework because of its electron deficiency. Computational studies suggest that extended boron sheets with partially filled hexagonal holes are stable; however, there has been no experimental evidence for such atom-thin boron nanostructures. Here, we show experimentally and theoretically that B36 is a highly stable quasiplanar boron cluster with a central hexagonal hole, providing the first experimental evidence that single-atom layer boron sheets with hexagonal vacancies are potentially viable. Photoelectron spectroscopy of B36− reveals a relatively simple spectrum, suggesting a symmetric cluster. Global minimum searches for B36− lead to a quasiplanar structure with a central hexagonal hole. Neutral B36 is the smallest boron cluster to have sixfold symmetry and a perfect hexagonal vacancy, and it can be viewed as a potential basis for extended two-dimensional boron sheets. Unlike carbon, boron is unable to form graphene-type structures, although variants with hexagonal holes have been suggested. Here the authors provide experimental evidence for the viability of such atom-thin boron sheets on the basis of a hexagonal vacancy discovered in a 36-atom planar boron cluster." @default.
• W2065575498 created "2016-06-24" @default.
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• W2065575498 date "2014-01-20" @default.
• W2065575498 modified "2023-10-16" @default.
• W2065575498 title "Planar hexagonal B36 as a potential basis for extended single-atom layer boron sheets" @default.
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• W2065575498 doi "https://doi.org/10.1038/ncomms4113" @default.
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