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- W2065595381 abstract "Synthetic methods that achieve oxidative 1,2-difunctionalization of alkenes are very powerful in organic chemistry. Here we report the first examples of intermolecular Pd-catalyzed aminoacetoxylation of alkenes with phthalimide as the nitrogen source and PhI(OAc)2 as the stoichiometric oxidant and source of acetate. These reactions are highly regio- and diastereoselective, and mechanistic studies reveal that the reaction proceeds via cis-aminopalladation of the alkene followed by oxidative cleavage of the intermediate Pd-C bond with inversion of stereochemistry." @default.
- W2065595381 created "2016-06-24" @default.
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- W2065595381 date "2006-05-09" @default.
- W2065595381 modified "2023-09-23" @default.
- W2065595381 title "Highly Regioselective Pd-Catalyzed Intermolecular Aminoacetoxylation of Alkenes and Evidence for <i>cis</i>-Aminopalladation and S<sub>N</sub>2 C−O Bond Formation" @default.
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- W2065595381 doi "https://doi.org/10.1021/ja061706h" @default.
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