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- W2065791749 abstract "A frequency doubled, tunable dye laser has been used to excite SO2 fluorescence in the region ≈2600–3200 Å. Two different groups of rovibronic states, having different zero pressure lifetimes and bimolecular quenching rates, are observed throughout the first excited singlet. The principal group of states has unusually long (≈80–600 μsec) collision free lifetimes, with bimolecular quenching rates and collision free lifetimes both decreasing to shorter excitation wavalenghts. The second group has a bimolecular quenching rate an order of magnitude above gas kinetic, and has not been observed by previous workers. A vibrational cascading non-exponentially effect in the decay of the principal group, first observed by Calvert and coworkers, has been confirmed. It is concluded that the unexpectedly long lifetimes and double exponential decay invalidate the conclusion of previous workers that SO2 undergoes a unimolecular internal conversion." @default.
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- W2065791749 date "1973-08-01" @default.
- W2065791749 modified "2023-09-23" @default.
- W2065791749 title "Collision free, time resolved fluorescence of SO2 excited near 2900 Å" @default.
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- W2065791749 doi "https://doi.org/10.1016/0009-2614(73)80135-6" @default.
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