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- W2065815636 abstract "Superphanes consisting of one thiophene ring and various substituted RCo-stabilized cyclobutadiene (CBD) rings (R = Cp, C5H4(CH3), C5(CH3)5, C5H4(Si(CH3)3), C5H4(COCH3), 8−12) and one superphane with one thiophene ring and one CpCo-stabilized cyclopentadienone ring (13) were synthesized. The starting point was a tricyclic diyne with a central thiophene ring and two condensed 4-cyclodecynes, 19. Heating of 19 with RCo(COD) yielded 8−12, whereas the heating of 19 with CpCo(CO)2 gave 13. X-ray structural investigation of 8−13 afforded the geometrical parameters in the solid state. Cyclic voltammetry showed a strong interaction between the thiophene ring and the CpCo-stabilized cyclobutadiene part. This interaction was substantiated by comparison between the CV data of 8−12 and model systems containing only the CpCo(CBD) part." @default.
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- W2065815636 date "2007-01-01" @default.
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- W2065815636 title "Transannular Interactions in Mixed Superphanes with One Thiophene and One CpCo-Stabilized Cyclobutadiene Ring: Syntheses, Structures, and Electrochemistry" @default.
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- W2065815636 doi "https://doi.org/10.1021/om0608206" @default.
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