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- W2066061161 abstract "The behavior of coherent field-induced hybrids of field-free rotor states (``pendular states'') is studied in energy regions where intramolecular vibrational energy redistribution phenomena are important. The energy region corresponding to the $4{ensuremath{nu}}_{1}$ band system of HCCF molecules, at approximately $12800{mathrm{cm}}^{ensuremath{-}1}$, has been chosen as an example. The calculations show that the expectation value of the orientation of molecules prepared in nonstationary pendular bright states exhibits a slow decay to the equilibrium value. Therefore the molecules substantially conserve their initial orientation after intramolecular vibrational redistribution takes place." @default.
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- W2066061161 date "1999-04-05" @default.
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- W2066061161 title "Pendular States of Highly Vibrationally Excited Molecules" @default.
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- W2066061161 doi "https://doi.org/10.1103/physrevlett.82.2856" @default.
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