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• W2066207825 abstract "By applying the concept of extended groups to the internal rotation problem in molecules with unequal halves, it has proved possible to construct a consistent formalism involving groups which correspond to very high, but finite multiples of the original Longuet-Higgins permutation-inversion group of the molecule. This formalism thus bridges the gap between the infinite extended groups used for linear molecules and the double groups used for molecules with two identical coaxial rotors. For the example of CF3NO considered explicitly in this paper, with permutation-inversion group isomorphic to C3v, the extended group is found to be isomorphic to C3m,v, where m is an integer obtained from the rational number pm which equals within experimental error the ratio ρ of top and molecule moments-of-inertia frequently introduced in discussions of the internal rotation problem. The extended group formalism can be used to rederive in an interesting fashion many results already well known from theoretical discussions in the earlier infrared and microwave literature, and shows promise for the treatment of as yet unsolved problems in molecules exhibiting internal rotation." @default.
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• W2066207825 date "1983-04-01" @default.
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• W2066207825 title "The application of extended permutation-inversion groups to internal rotation of a symmetric rotor top in a symmetric or asymmetric rotor molecule" @default.
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• W2066207825 doi "https://doi.org/10.1016/0022-2852(83)90249-7" @default.
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