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• W2066413890 abstract "We report the investigation of surface forces between polyelectrolyte multilayers of poly(allylamine hydrochloride) (PAH) and poly(styrenesulfonate sodium salt) (PSS) assembled on mica surfaces during film buildup using a surface force apparatus. Up to four polyelectrolyte layers were prepared on each surface ex situ, and the surface interactions were measured in 10-4 M KBr solutions. The film thickness under high compressive loads (above 2000 μN/m) increased linearly with the number of deposited layers. In all cases, the interaction between identical surfaces at large separations (>100 Å from contact) was dominated by electrostatic double-layer repulsion. By fitting DLVO theory to the experimental force curves, the apparent double-layer potential of the interacting surfaces was calculated. At shorter separations, an additional non-DLVO repulsion was present due to polyelectrolyte chains extending some distance from the surface into solution, thus generating an electrosteric type of repulsion. Forces between dissimilar multilayers (i.e., one of the multilayers terminated with PSS and the other with PAH) were attractive at large separations (30−400 Å) owing to a combination of electrostatic attraction and polyelectrolyte bridging." @default.
• W2066413890 created "2016-06-24" @default.
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• W2066413890 date "2004-05-18" @default.
• W2066413890 modified "2023-10-03" @default.
• W2066413890 title "Surface Interactions during Polyelectrolyte Multilayer Buildup. 1. Interactions and Layer Structure in Dilute Electrolyte Solutions" @default.
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• W2066413890 doi "https://doi.org/10.1021/la049636k" @default.
• W2066413890 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/15986683" @default.
• W2066413890 hasPublicationYear "2004" @default.
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