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- W2066455071 abstract "We investigate harmonic generation from $text{H}_{2}{}^{+}$ molecules driven by intense few-cycle laser pulses whose linearly polarization axis makes an arbitrary angle $ensuremath{chi}$ with respect to the molecular axis. The $text{H}_{2}{}^{+}$ molecule is considered initially in various orbitals with nodal planes. It is found that a strong enhancement of high-order harmonics (HOHs) occurs when the laser polarization axis overlaps with major axes of electron distribution in the active orbital, while broad suppression of HOHs occurs when the laser polarization axis is parallel to a nodal plane of the active molecular orbital. We show that this harmonic suppression is enhanced by destructive interferences when the nodal and the laser polarization axes are parallel to the internuclear axis, which leads to a shortening of the harmonic cutoff. It follows that the orientation dependence of HOHs intensities mimics the electronic density in active orbitals through the angular dependence of ionization and recombination processes." @default.
- W2066455071 created "2016-06-24" @default.
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- W2066455071 date "2009-10-12" @default.
- W2066455071 modified "2023-09-25" @default.
- W2066455071 title "Orbital symmetry and interference effects in molecular high-order harmonic generation" @default.
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- W2066455071 doi "https://doi.org/10.1103/physreva.80.041403" @default.
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