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- W2066524319 abstract "The author analyzes the mutual influence of temperature variation and mass transfer in a model absorption system. The latter consists of a free laminar jet of liquid surrounded by gaseous atmosphere. At the inlet the liquid contains species A dissolved in it. Gas B which is absorbed through the exposed surfaces, dissolves in the liquid, and then undergoes irreversible chemical reaction of the second or higher order with A. It is assumed that the reaction rate is equal to a rate constant times the product of the concentrations of the species raised to certain powers. The rate constant is a monotonically increasing function of the temperature, while the chemical reaction tends to lower or raise the temperature of the liquid with respect to its ambient level. On the other hand, these temperature changes influence the reaction process. Evidently, solutions which exhibit distinctly different behaviors are possible. The coupling between the mass and the heat transfer mechanisms is demonstrated by constructing only two cases. In Case (i) the reaction rate is taken to be small at the ambient temperature and also not too sensitive to temperature changes. For such a case the coupling is relatively weak, particularly if the free surfaces are maintained at the ambient temperature. The coupling is stronger if the free surfaces are thermally insulated and consequently there is a more significant change in the temperature of the liquid. The coupling is very strong in Case (ii), when the reaction rate is taken to be a sensitive function of the temperature and the chemical reaction is assumed to be highly exothermic. The solutions presented are obtained by the method of singular perturbations. In Case (i) the singularity is associated with the infinite nature of the domain. To Case (ii) there is a boundary — or rather ‘reaction layer’ type of solution." @default.
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- W2066524319 date "1973-07-01" @default.
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- W2066524319 title "Combined heat and mass transfer for two reacting species with temperature dependent reaction constant" @default.
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- W2066524319 doi "https://doi.org/10.1016/0009-2509(73)85151-6" @default.
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