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• W2066671723 abstract "Measurements of dielectric constant as a function of temperature give clear evidence of molecular rotation in many crystalline phases comparable to the rotation in liquids and in a few organic glasses which have been studied. The effect of molecular shape upon rotation is examined, it being shown that spheroidal and cylindrical molecules may rotate. The rotation may be presumed usually to consist of rotational jumps between potential energy minima. Rotational freedom depends upon the closeness of the approach to one of the ratios of the molecular radii in different directions, but is influenced by the closeness of the molecular packing. Many solids which show a rotational transition point are soft, waxy, and translucent in this rotator phase between the transition point and the melting-point and brittle below the transition point. A number of solids which show anomalous dielectric dispersion like that found in liquids and organic glasses, but no rotational transition, are brittle. It appears that plasticity may result from the increase in volume per molecule occurring when slightly unsymmetrical molecules begin to rotate at a transition point. Dielectric relaxation measurements show that the internal friction resisting molecular rotation in the crystal is, in some cases, about the same as in the liquid state, and, in some cases, much less." @default.
• W2066671723 created "2016-06-24" @default.
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• W2066671723 date "1961-01-01" @default.
• W2066671723 modified "2023-09-26" @default.
• W2066671723 title "Dielectric evidence of molecular rotation in solids∗" @default.
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• W2066671723 doi "https://doi.org/10.1016/0022-3697(61)90081-6" @default.
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