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• W2066704740 startingPage "1384" @default.
• W2066704740 abstract "It is shown that a mapping of precomputed rate data can be used to implement efficiently detailed surface mechanisms into reactor simulations. The procedure is demonstrated using a surface mechanism for CH4 oxidation on platinum (11 surface species, 19 reactions). It is found that a spline representation based on 7000 data points reproduces the effective CH4 conversion rates with an error of less than 0.5%. To demonstrate the potential of the approach a 3D model of a monolith channel including the irregularly shaped washcoat is implemented in a commercial CFD program. A steady state solution of this model takes 20 s on a 1.5 GHz Pentium computer. This corresponds to a speed up of three orders of magnitude compared to the solution of the same model coupled to a full numerical solution of the surface chemistry." @default.
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• W2066704740 date "2009-04-01" @default.
• W2066704740 modified "2023-10-02" @default.
• W2066704740 title "Efficient implementation of detailed surface chemistry into reactor models using mapped rate data" @default.
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• W2066704740 doi "https://doi.org/10.1016/j.ces.2008.12.006" @default.
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