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• W2066765497 abstract "CuI and CuII coordination polymers of 1,10-dithia-18-crown-6 (L) with unusual networking modes involving an exocyclic coordination are presented. The reaction of L with copper(II) nitrate gave a unprecedented ladder-type 1D coordination polymer {[(LOXOX)Cu2(NO3)2(H2O)4](LOXOX)(NO3)2·2H2O}n (1) via strong CuII–Osulfoxide bonds because L was oxidized to the disulfoxide macrocycle (LOXOX) under the present conditions. Meanwhile the parallel reaction of copper(I) iodide with L in the presence of cobalt(II) perchlorate yielded a mixture of an emissive 2D network product [(Cu4I4)(L)2]n (2) linked with cubane-type Cu4I4 clusters and a non-emissive 1D coordination polymer {[(Cu2I2)(L)2][Co(H2O)6](ClO4)2·0.5H2O}n (3) linked with rhomboidal Cu2I2 cores. In 3, hexaaquacobalt(II) complexes, anions and water molecules also exist and stabilize the 1D macrocyclic network through H-bonds." @default.
• W2066765497 created "2016-06-24" @default.
• W2066765497 creator A5024061112 @default.
• W2066765497 creator A5074243341 @default.
• W2066765497 date "2011-01-01" @default.
• W2066765497 modified "2023-09-27" @default.
• W2066765497 title "Networking of macrocycles: 1D and 2D coordination polymers of dithia-18-crown-6 with copper(ii) and copper(i)" @default.
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• W2066765497 doi "https://doi.org/10.1039/c1ce05587a" @default.
• W2066765497 hasPublicationYear "2011" @default.
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