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• W2066887117 endingPage "1295" @default.
• W2066887117 startingPage "1261" @default.
• W2066887117 abstract "Abstract We design a circularly polarized laser pulse in the infrared frequency and femtosecond time domains, for excitation of the OsH 4 molecule in its first excited pseudorotational state of the triply‐degenerate bend. The OsH 4 molecule need not be pre‐oriented. After excitation, the central nucleus Os carries out pseudorotation about the axis parallel to the direction of propagation of the laser pulse. This pseudorotation causes a strong electric ring current with a value I =1.53 e fs −1 . The mean value of the radius of the ring current is very small, R =0.0031 a 0 , where a 0 is the Bohr radius. According to the Biot–Savart law (| ${{vec{bf B}}}$ ( R = 0 )|∼ I / R ), this nuclear ring current induces the strongest magnetic field predicted so far in molecules, with a central peak absolute value | ${{vec{bf B}}}$ ( R = 0 )|=623 T. To monitor the effect, we propose an IR‐pump–X‐ray‐probe versus an X‐ray‐probe‐only experiment, at the K‐ and L ‐edges of X‐ray ionization. The results are based on the general quantum theory of excitations of pseudorotations in tetrahedral molecules AB 4 , driven by a circularly polarized laser pulse." @default.
• W2066887117 created "2016-06-24" @default.
• W2066887117 creator A5000707265 @default.
• W2066887117 creator A5040547033 @default.
• W2066887117 creator A5044928380 @default.
• W2066887117 creator A5054582897 @default.
• W2066887117 date "2012-03-02" @default.
• W2066887117 modified "2023-10-18" @default.
• W2066887117 title "Strong Nuclear Ring Currents and Magnetic Fields in Pseudorotating OsH₄Molecules Induced by Circularly Polarized Laser Pulses" @default.
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• W2066887117 doi "https://doi.org/10.1002/asia.201100776" @default.
• W2066887117 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22389250" @default.

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