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- W2066932912 abstract "The vibrational coupling in the ground and excited states of positively charged naphthalene, anthracene, tetracene, and pentacene molecules is studied on the basis of a joint experimental and theoretical study of ionization spectra using high-resolution gas-phase photoelectron spectroscopy and first-principles correlated quantum-mechanical calculations. Our theoretical and experimental results reveal that, while the main contribution to relaxation energy in the ground state of oligoacene systems comes from high-energy vibrations, the excited-state relaxation energies show a significant redistribution toward lower-frequency vibrations. A direct correlation is found between the nature of the vibronic interaction and the pattern of the electronic state structure." @default.
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- W2066932912 date "2006-06-13" @default.
- W2066932912 modified "2023-10-17" @default.
- W2066932912 title "Vibronic Coupling in the Ground and Excited States of Oligoacene Cations" @default.
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- W2066932912 doi "https://doi.org/10.1021/jp057462p" @default.
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