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• W2067036723 abstract "Highly pure semiconducting single-walled carbon nanotubes (SWNTs) are essential for the next generation of electronic devices, such as field-effect transistors and photovoltaic applications; however, contamination by metallic SWNTs reduces the efficiency of their associated devices. Here we report a simple and efficient method for the separation of semiconducting- and metallic SWNTs based on supramolecular complex chemistry. We here describe the synthesis of metal-coordination polymers (CP-Ms) composed of a fluorene-bridged bis-phenanthroline ligand and metal ions. On the basis of a difference in the ‘solubility product’ of CP-M-solubilized semiconducting SWNTs and metallic SWNTs, we readily separated semiconducting SWNTs. Furthermore, the CP-M polymers on the SWNTs were simply removed by adding a protic acid and inducing depolymerization to the monomer components. We also describe molecular mechanics calculations to reveal the difference of binding and wrapping mode between CP-M/semiconducting SWNTs and CP-M/metallic SWNTs. This study opens a new stage for the use of such highly pure semiconducting SWNTs in many possible applications. Semiconducting single-wall nanotubes hold promise for the next generation of electronic devices, but separating them from metallic counterparts is still challenging. Here, the authors show how to sort semiconducting nanotubes by selectively stabilizing them in solution via a removable solubilizer." @default.
• W2067036723 created "2016-06-24" @default.
• W2067036723 creator A5005651563 @default.
• W2067036723 creator A5068533962 @default.
• W2067036723 date "2014-10-03" @default.
• W2067036723 modified "2023-10-02" @default.
• W2067036723 title "Semiconducting single-walled carbon nanotubes sorting with a removable solubilizer based on dynamic supramolecular coordination chemistry" @default.
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• W2067036723 doi "https://doi.org/10.1038/ncomms6041" @default.
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