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- W2067126405 abstract "The active role of the optically dark pi sigma* state, following UV absorption, has been implicated in the photochemistry of a number of biomolecules. This work focuses on the role of the pi sigma* state in the photochemistry of phenol upon excitation at 200 nm. By probing the neutral hydrogen following UV excitation, we show that hydrogen elimination along the dissociative pi sigma* potential energy surface occurs within 103 +/- 30 fs, indicating efficient coupling at the S1/S2 and S0/S2 conical intersections, with no identifiable role of statistical unimolecular decay of vibronically excited (S0) phenol in the timeframe of our measurements." @default.
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- W2067126405 date "2008-06-10" @default.
- W2067126405 modified "2023-10-16" @default.
- W2067126405 title "Direct versus Indirect H Atom Elimination from Photoexcited Phenol Molecules" @default.
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- W2067126405 doi "https://doi.org/10.1021/jp802155b" @default.
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