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• W2067245318 endingPage "2971" @default.
• W2067245318 startingPage "2968" @default.
• W2067245318 abstract "Gas-phase synthesized vanadium−benzene 1:2 (VBz2) sandwich clusters were size-selectively deposited onto bare gold and long-chain n-alkanethiolate [−S−(CH2)n-1−CH3; n = 16, 18, and 22] self-assembled monolayer (SAM)-coated gold substrates under ultrahigh vacuum (UHV) conditions. Investigation of the resulting deposited clusters was performed by infrared reflection absorption spectroscopy (IRAS) and thermal desorption spectroscopy (TDS). The IR frequencies of the soft-landed VBz2 clusters show excellent agreement with the fundamentals reported in IR data of VBz2 in an argon matrix. The analysis of IRAS spectra reveals that while there was no orientational preference of the VBz2 clusters on a bare gold substrate, the VBz2 clusters deposited onto the SAM substrates were highly oriented with the molecular axis 70−80° tilted off the surface normal. In addition, analysis of TDS spectra revealed unusually large adsorption heats of the physisorbed VBz2 clusters. The present results are explained by cluster penetration into the long-chain alkanethiolate SAM and for the first time demonstrate the matrix isolation of gas-phase organometallic clusters around room temperature." @default.
• W2067245318 created "2016-06-24" @default.
• W2067245318 creator A5036540267 @default.
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• W2067245318 date "2006-02-01" @default.
• W2067245318 modified "2023-09-27" @default.
• W2067245318 title "Soft-Landing Isolation of Vanadium−Benzene Sandwich Clusters on a Room-Temperature Substrate Using <i>n</i>-Alkanethiolate Self-Assembled Monolayer Matrixes" @default.
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• W2067245318 doi "https://doi.org/10.1021/jp057194v" @default.
• W2067245318 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16494294" @default.
• W2067245318 hasPublicationYear "2006" @default.
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