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- W2067382772 abstract "A new heterometallic dyad composed of a zinc porphyrin linked by bisethynyl quaterthiophene to a gold porphyrin was synthesized according to a stepwise modular approach. The latter dyad and the parent reference compounds (porphyrin-ethynylquaterthiophene) were characterized by electrochemistry, spectroelectrochemistry, and femtosecond transient absorption spectrocopy. We showed that light excitation of the zinc or the gold porphyrin induces a very fast and quantitative charge separation over a distance of 25 Å which occurs through a superexchange mechanism. The lifetime of the charge-separated state is 3.3 ns in toluene and 100 ps in dichloromethane, and it recombines to the ground state in both solvents." @default.
- W2067382772 created "2016-06-24" @default.
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- W2067382772 date "2008-12-12" @default.
- W2067382772 modified "2023-10-04" @default.
- W2067382772 title "Very Fast Single-Step Photoinduced Charge Separation in Zinc Porphyrin Bridged to a Gold Porphyrin by a Bisethynyl Quaterthiophene" @default.
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- W2067382772 doi "https://doi.org/10.1021/ic800727e" @default.
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