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- W2067476211 abstract "We present a theory of the autoacceleration of polymerization rates during free radical polymerization, known as the gel effect. Termination reactions between long living chains are so retarded by entanglements that short-long terminations provide the fastest mechanism. Consistent with several experiments, this leads to polymerization rates independent of the radical production rate ${R}_{i}$, in contrast to the $sqrt{{R}_{i}}$ dependence in the classical theory. For long chains, the instantaneous polymer product is a copy of the living population, following an exponential distribution with mean length $overline{N}ensuremath{sim}frac{1}{{R}_{i}}$." @default.
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- W2067476211 date "1994-09-19" @default.
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- W2067476211 title "Autoacceleration in Free Radical Polymerization" @default.
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- W2067476211 doi "https://doi.org/10.1103/physrevlett.73.1723" @default.
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