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• W2067587058 abstract "The cubic electron-spin-resonance spectrum of ${mathrm{Fe}}^{3+}$ in silver chloride has been studied at 1.3ifmmode^circelsetextdegreefi{}K by the electron-nuclear-double-resonance (ENDOR) technique. ENDOR lines from 6 to 24 Mc/sec were observed on each of the five electron-spin-resonance transitions and have been identified as lines due to four chlorine nuclei which are nearest neighbors to the iron ion. The angular dependence of the crystal-field splitting of the electron resonance, as the orientation of the applied field is varied, proves that the iron is in a site of cubic symmetry. The angular variation of the ENDOR spectrum, as the field is rotated in a (100) plane, shows that the iron cannot be in a site of octahedral symmetry and that it therefore must be in a site of tetrahedral symmetry. ENDOR lines of both chlorine isotopes were identified. ${mathrm{Cl}}^{35}$ ENDOR lines, chartetrahedral by ${M}_{s}=+frac{3}{2}$ and ${M}_{s}=ensuremath{-}frac{3}{2}$, were studied with the applied field parallel to the [100] direction, and the best chlorine hyperfine and quadrupole coupling constants were determined for both isotopes. It is found that these constants can be used to predict the locations of all observed ${mathrm{Cl}}^{35}$ and ${mathrm{Cl}}^{37}$ ENDOR lines, but some discrepancies between the predicted spectrum and the observed lines remain which cannot be accounted for by effects of the cubic-field splitting term in the spin Hamiltonian." @default.
• W2067587058 created "2016-06-24" @default.
• W2067587058 creator A5026444322 @default.
• W2067587058 date "1965-10-18" @default.
• W2067587058 modified "2023-10-09" @default.
• W2067587058 title "Magnetic-Resonance Study of Iron in Silver Chloride" @default.
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• W2067587058 doi "https://doi.org/10.1103/physrev.140.a656" @default.
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