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• W2067652094 abstract "In the mid-1990s, a groundwater plume of uranium (U) was detected in monitoring wells in the B-BX-BY Waste Management Area at the Hanford Site in Washington. This area has been used since the late 1940s to store high-level radioactive waste and other products of U fuel-rod processing. Using multiple-collector ICP source magnetic sector mass spectrometry, high-precision uranium isotopic analyses were conducted of samples of vadose zone contamination and of groundwater. The isotope ratios 236U/238U, 234U/238U, and 238U/235U are used to distinguish contaminant sources. On the basis of the isotopic data, the source of the groundwater contamination appears to be related to a 1951 overflow event at tank BX-102 that spilled high-level U waste into the vadose zone. The U isotopic variation of the groundwater plume is a result of mixing between contaminant U from this spill and natural background U. Vadose zone U contamination at tank B-110 likely predates the recorded tank leak and can be ruled out as a significant source of groundwater contamination, based on the U isotopic composition. The locus of vadose zone contamination is displaced from the initial locus of groundwater contamination, indicating that lateral migration in the vadose zone was at least 8 times greater than vertical migration. The time evolution of the groundwater plume suggests an average U migration rate of ∼0.7−0.8 m/day showing slight retardation relative to a groundwater flow of ∼1 m/day." @default.
• W2067652094 created "2016-06-24" @default.
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• W2067652094 date "2004-05-18" @default.
• W2067652094 modified "2023-09-27" @default.
• W2067652094 title "Identifying the Sources of Subsurface Contamination at the Hanford Site in Washington using High-Precision Uranium Isotopic Measurements" @default.
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• W2067652094 doi "https://doi.org/10.1021/es034700q" @default.
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