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- W2067996846 abstract "Abstract We show that BiB 3 O 6 (BiBO) crystals, well known for their excellent second harmonic generation (SHG) properties, may also be of interest for third-order optical phenomena, particularly for two-photon absorption (TPA). Photoinduced TPA measurements were performed under illumination of excimer Xe–F laser ( λ = 217 nm) as a photoinducing (pumping) beam. It created a thin surface layer (about 85 nm) that was a source of the observed photoinduced TPA. Raman shifted Nd-YAG laser radiation ( λ = 1.9 μm) as well as its second and fourth harmonics ( λ = 950 and λ = 475 nm, respectively) were used as fundamental (probing) beams of the TPA. The highest values of the TPA β coefficient were achieved for a polarization of the pumping light directed along crystallographic axis b . Quantum chemical simulations indicate on substantial contribution of UV-induced electron–phonon anharmonicity to the observed TPA. The obtained values of TPA coefficients indicate a possibility of using BiBO crystals as UV-operated optical limiters in a wide spectral range." @default.
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- W2067996846 date "2005-06-01" @default.
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- W2067996846 title "UV-induced two-photon absorption in BiB3O6 single crystals" @default.
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- W2067996846 doi "https://doi.org/10.1016/j.optcom.2005.02.053" @default.
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