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• W2068263124 startingPage "L929" @default.
• W2068263124 abstract "For the first time the symmetric bending vibrational frequencies (v2) of NH3 physisorbed on a partially hydroxylated metal oxide surface have been obtained with the coherent anti-Stokes Raman spectroscopy (CARS) using the planar optical waveguide geometry. The CARS signal from the adsorbed NH3 was enhanced by establishing an interference condition within the waveguide to reduce the CARS contribution from the oxide surface. The surface CARS spectra, in the investigated v2 spectral region, provided evidence that the partially hydroxylated ZnO surface supported several sites for the physisorption of NH3. The physisorbed species had v2 frequencies around 950, 963, 975 and 1012 cm−1 and were very quickly desorbed as soon as evacuation of the vacuum chamber began. In addition, the presence of NH3 which is coordinated to Zn2+ sites on the surface was detected." @default.
• W2068263124 created "2016-06-24" @default.
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• W2068263124 date "1993-09-01" @default.
• W2068263124 modified "2023-09-27" @default.
• W2068263124 title "Direct observation of the symmetric bending vibrations (v2) of NH3 physisorbed on a partially hydroxylated planar (0001) surface of ZnO" @default.
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• W2068263124 doi "https://doi.org/10.1016/0039-6028(93)90150-i" @default.
• W2068263124 hasPublicationYear "1993" @default.
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