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- W2068449944 abstract "Fluctuations of enthalpy and density in the isostress-isostrain ensemble are employed to accumulate evidence for shear strain induced melting (shear melting) to occur as a second order liquid-solid phase transition. Shear melting of a solid-like monolayer film in a model slit-pore (vicinal phase) is studied by means of an isostress-isostrain ensemble Monte Carlo (MC) method. Quantities of prime interest are isostress heat capacity c 3, isothermal compressibility χ3 and isostress expansivity γ3 where the subscript ‘3’ references the component of stress normal to the pore walls. If studied as functions of laterally applied strain α, these quantities diverge at the shear melting point αc according to theoretical considerations. Theory also predicts a power law decay of c 3, χ3 and γ3 proportional to (α - αc) v for α > αc where v is a critical exponent. Fitting the power law to MC data for c 3 yields αc = 0·28 in very good agreement with previous structural and dynamic results for the same thermodynamic state. Our results do not show any significant system size dependence. Average film thickness depends solely on thermodynamic conditions and not on enlarging the pore cross-section in the (x, y) plane. The same can be expected for fluctuations around this average value. Although fluctuations of enthalpy and density diverge at αc, enthalpy and density themselves remain continuous functions of applied strain everywhere. Thus, shear melting occurs without release of latent heat, which furnishes further evidence for a liquid-solid phase transition of second order." @default.
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- W2068449944 date "1993-04-10" @default.
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- W2068449944 title "Isostress-isostrain ensemble Monte Carlo simulation of second order phase transitions in a confined monolayer fluid" @default.
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