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- W2068503825 abstract "Experimental results have been obtained which show that carbon formation in ethanol-air diffusion flames occurs preferentially from the nonhydroxylated carbon atom of the ethanol molecule. The ratio of the contribution to solid carbon of the nonhydroxylated carbon atom to that of the hydroxylated atom equals 2:1. These findings support a proposed carbon formation mechanism, which is based on previous experimental observations and theoretical considerations. In order to define the overall reaction paths of each of the carbon atoms a radioisotopic tracer technique is developed. Ethanol-1-14C and ethanol-2-14C fuels are burned in a specially designed diffusion burner, and the radioactivities of collected samples of solid carbon are measured. A comparative analysis of the specific activities of the fuels and carbon samples defines the contribution of each of the carbon atoms to solid carbon. The technique proves to be a useful, quantitative tool for carbon formation research. In addition to the well-defined conclusions of the investigation, the particular numerical results suggest that carbon formation may be controlled by the selective one-to-one addition of two- and one-carbon fragments present in the flame—a new and intriguing explanation of the carbon formation pnenomenon. This novel suggestion is discussed in light of the present and previous experimental observations." @default.
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- W2068503825 date "1970-06-01" @default.
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- W2068503825 title "A radioisotopic tracer study of carbon formation in ethanol-air diffusion flames" @default.
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- W2068503825 doi "https://doi.org/10.1016/s0010-2180(70)80042-6" @default.
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