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• W2068514557 abstract "High-resolution $^{77}text{S}text{e}$ nuclear magnetic resonance spectroscopy is used to investigate the rotational dynamics of Se atoms in ${text{Ge}}_{x}{text{Se}}_{100ensuremath{-}x}$ supercooled liquids with $5ensuremath{le}xensuremath{le}23$. The Se atoms in Se-Se-Se linkages are found to be significantly more mobile compared to those in Ge-Se-Se/Ge linkages. The time scale of the rotational dynamics of Se-Se-Se linkages and its temperature dependence are nearly identical for liquids with $xensuremath{le}17$ but the time scale displays an abrupt increase for the liquids with $x=20$ and 23, at and above the rigidity percolation threshold. Such a dynamical transition is shown to be consistent with a sudden elastic stiffening of the atomic network of ${text{Ge}}_{x}{text{Se}}_{100ensuremath{-}x}$ supercooled liquids at the percolation threshold." @default.
• W2068514557 created "2016-06-24" @default.
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• W2068514557 date "2010-07-26" @default.
• W2068514557 modified "2023-09-27" @default.
• W2068514557 title "Mechanistic understanding of the effect of rigidity percolation on structural relaxation in supercooled germanium selenide liquids" @default.
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• W2068514557 doi "https://doi.org/10.1103/physrevb.82.014203" @default.
• W2068514557 hasPublicationYear "2010" @default.
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