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- W2068682621 abstract "The chemical composition and dissociation behaviour of water adsorbed on clean and oxygen pre-covered Pd{1 1 1} was studied using high-resolution time-resolved and temperature-programmed X-ray photoelectron spectroscopy. We find that water remains intact at all temperatures up to desorption on the clean surface and at high oxygen coverage(0.69 ML) when a surface oxide is formed. The highest desorption peaks occur at 163 K from the clean surface and at 172 K from the surface oxide. At the intermediate coverage of 0.20 ML oxygen reacts with coadsorbed water at 155 K, to generate a mixed H2O/OH layer exhibiting a (3×3)R30° diffraction pattern, which is stable up to 177 K. The measured ratio between intact water and the hydroxyl species in this layer varies between 1.5 and 2 depending on temperature." @default.
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- W2068682621 date "2008-11-01" @default.
- W2068682621 modified "2023-10-18" @default.
- W2068682621 title "Chemical composition and reactivity of water on clean and oxygen-covered Pd{111}" @default.
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- W2068682621 doi "https://doi.org/10.1016/j.susc.2008.09.031" @default.
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