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• W2068876997 abstract "A novel series of solid-solution semiconductors (AgNbO3)1−x(SrTiO3)x (0 ≤ x ≤ 1) have been developed as highly visible-light-active photocatalysts for efficient O2 evolution and decomposition of organic pollutants. Rietveld refinement reveals that the perovskite-type solid solutions (AgNbO3)1−x(SrTiO3)x are crystallized in an orthorhombic system (0 ≤ x < 0.9) or a cubic system (0.9 ≤ x ≤ 1). In the mixed valent perovskites (AgNbO3)1−x(SrTiO3)x, the hybridization behaviors between the Ag 4d and O 2p orbitals and between the Nb 4d and Ti 3d orbitals play a crucial role in tuning the energy band structure (band gap, band edge, and bandwidth, etc.) and, thus, in tailoring the photophysical and photocatalytic properties. As a result of competition between the absorption ability to visible-light and the reductive/oxidative abilities, the highest visible-light activities for both O2 evolution and decomposition of gaseous 2-propanol (IPA) are realized over (AgNbO3)0.75(SrTiO3)0.25. In addition, very fine Ag parti..." @default.
• W2068876997 created "2016-06-24" @default.
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• W2068876997 date "2009-02-06" @default.
• W2068876997 modified "2023-10-11" @default.
• W2068876997 title "New Series of Solid-Solution Semiconductors (AgNbO₃)_1−<i>x</i>(SrTiO₃)_<i>x</i> with Modulated Band Structure and Enhanced Visible-Light Photocatalytic Activity" @default.
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• W2068876997 doi "https://doi.org/10.1021/jp807393a" @default.
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