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- W2069063124 abstract "A new mechanism has been presented for the vibrational mode-specific depression of the proton-transfer reaction NH3+ (ν) + NH3 → NH2 + NH4+. We adopt the standpoint of the ADO (average dipole orientation) theory, proposed by Su and Bowers (J. Chem. Phys. 58 (1973) 3027), and append a new long-range interaction created by a vibration-induced dipole to the ADO theory. A “reaction zone” concept is crucial in this approach; outside of the zone the long-range intermolecular interactions play a key role. A qualitatively good agreement is observed for the experimental result of the title reaction obtained by Chupka and Russel (J. Chem. Phys. 48 (1968) 1527)." @default.
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- W2069063124 date "1991-09-01" @default.
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- W2069063124 title "New mechanism for the vibrational mode-specific proton-transfer reaction NH3+ (ν) + NH3 → NH2 + NH4+" @default.
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- W2069063124 doi "https://doi.org/10.1016/0301-0104(91)87039-x" @default.
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