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- W2069094014 abstract "A Cu–carborane-based metal–organic framework (MOF), NU-135, which contains a quasi-spherical para-carborane moiety, has been synthesized and characterized. NU-135 exhibits a pore volume of 1.02 cm3/g and a gravimetric BET surface area of ca. 2600 m2/g, and thus represents the first highly porous carborane-based MOF. As a consequence of the unique geometry of the carborane unit, NU-135 has a very high volumetric BET surface area of ca. 1900 m2/cm3. CH4, CO2, and H2 adsorption isotherms were measured over a broad range of pressures and temperatures and are in good agreement with computational predictions. The methane storage capacity of NU-135 at 35 bar and 298 K is ca. 187 vSTP/v. At 298 K, the pressure required to achieve a methane storage density comparable to that of a compressed natural gas (CNG) tank pressurized to 212 bar, which is a typical storage pressure, is only 65 bar. The methane working capacity (5–65 bar) is 170 vSTP/v. The volumetric hydrogen storage capacity at 55 bar and 77 K is 49 g/L. T..." @default.
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- W2069094014 date "2013-08-22" @default.
- W2069094014 modified "2023-10-18" @default.
- W2069094014 title "Carborane-Based Metal–Organic Framework with High Methane and Hydrogen Storage Capacities" @default.
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- W2069094014 doi "https://doi.org/10.1021/cm4020942" @default.
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