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- W2069133367 abstract "A general theory is presented for the long-range behavior of the pair-correlation function in a multi-component mixture, based on the thermodynamics of inhomogeneous systems. A set of nonlinear, coupled differential equations are obtained for the correlation function, and these reduced to linear equations under well-defined approximations. When applied to a one-component system, it is found that previously proposed equations of Ornstein and Zernike, and Hart are included as special cases of the linear theory. The assumptions implicit in these equations are clarified. The theory has also been used to obtain an asymptotic solution for the pair-correlation functions of a binary mixture. The conditions under which these equations reduce to expressions similar to those for pure fluids are investigated." @default.
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- W2069133367 date "1968-12-15" @default.
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- W2069133367 title "General Theory of the Long-Range Pair-Correlation Function" @default.
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