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- W2069366831 abstract "The palladium-catalyzed telomerization of 1,3-butadiene with alcohols has been studied in presence of palladium and imidazolium salts, which form in situ carbene ligands. Among the different imidazolium salts tested 1,3-dimesitylimidazolium chloride (7), 1,3-bis(ferrocenylmethyl)benzimidazolium tetraphenylborate (12) and 1,3-bis(2-ferrocenylethyl)benzimidazolium bromide (13) gave the best yields of the desired octadienyl ethers. Significantly improved regioselectivities for the linear octadienylethers are obtained in the reaction of 1,3-butadiene and methanol compared to the previously optimized palladium/triphenylphosphine catalyst. Using n-butanol and iso-propanol the palladium carbene catalysts lead to a considerable increase in the corresponding telomerization products compared to standard palladium/triphenylphosphine catalysts." @default.
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- W2069366831 date "2002-07-01" @default.
- W2069366831 modified "2023-10-14" @default.
- W2069366831 title "Efficient telomerization of 1,3-butadiene with alcohols in the presence of in situ generated palladium(0)carbene complexes" @default.
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- W2069366831 doi "https://doi.org/10.1016/s1381-1169(02)00068-7" @default.
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